Inverted ITO- and PEDOT:PSS-free polymer solar cells with high power conversion efficiency
Identifieur interne : 000A11 ( Main/Repository ); précédent : 000A10; suivant : 000A12Inverted ITO- and PEDOT:PSS-free polymer solar cells with high power conversion efficiency
Auteurs : RBID : Pascal:13-0303789Descripteurs français
- Pascal (Inist)
- Addition étain, Cellule solaire organique, Rendement élevé, Grande puissance, Conversion énergie, Taux conversion, Palier, Couche ITO, Production industrielle, Processus fabrication, Procédé fabrication, Structure flexible, Diminution coût, Empilement, Addition aluminium, Cellule solaire, Hétérojonction, Résistivité couche, Compatibilité, Oxyde d'indium, Styrènesulfonate polymère, Thiophène dérivé polymère, Mélange polymère, Oxyde d'aluminium, Oxyde de zinc, Couche mince, Argent, Matériau transparent, ITO.
- Wicri :
- concept : Production industrielle, Argent.
English descriptors
- KwdEn :
- Aluminium addition, Aluminium oxide, Bearing(mechanics), Compatibility, Conversion rate, Cost lowering, Energy conversion, Flexible structure, Heterojunction, High efficiency, High power, ITO layers, Indium oxide, Industrial production, Manufacturing process, Organic solar cells, Polymer blends, Production process, Sheet resistivity, Silver, Solar cell, Stacking, Styrenesulfonate polymer, Thin film, Thiophene derivative polymer, Tin addition, Transparent material, Zinc oxide.
Abstract
Highest published power conversion efficiencies of organic solar cells have mostly been achieved on substrates bearing a transparent indium tin oxide (ITO) electrode. However, the incorporation of ITO is not suited for future industrial production processes of organic solar cells, which will rely on a high-throughput of flexible substrates in order to achieve low cost of the final product. In this manuscript we present an alternative transparent electrode consisting of a layer stack of aluminum doped zinc oxide and a thin silver layer. Substrates with these electrodes have a transparency of above 75% in the wavelength range in which the photoactive layer absorbs light. Solar cells with a bulk-heterojunction of PTB7 and PC71BM in an inverted device architecture achieved a power conversion efficiency of 6.1%, which is the highest reported value for polymer solar cells free from both ITO and PEDOT:PSS. The sheet resistance of the novel electrodes increased only marginally after repeated bending which shows their full compatibility with future reel-to-reel processes or flexible products.
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Pascal:13-0303789Le document en format XML
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aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Bade-Wurtemberg</region><region type="district" nuts="2">District de Fribourg-en-Brisgau</region><settlement type="city">Fribourg-en-Brisgau</settlement></placeName></affiliation></author><author><name sortKey="Grein, Maria" uniqKey="Grein M">Maria Grein</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstrasse 2</s1><s2>79110 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Bade-Wurtemberg</region><region type="district" nuts="2">District de Fribourg-en-Brisgau</region><settlement type="city">Fribourg-en-Brisgau</settlement></placeName></affiliation></author><author><name sortKey="Reinecke, Patrick" uniqKey="Reinecke P">Patrick Reinecke</name><affiliation wicri:level="3"><inist:fA14 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T">Thomas Kroyer</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstrasse 2</s1><s2>79110 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Bade-Wurtemberg</region><region type="district" nuts="2">District de Fribourg-en-Brisgau</region><settlement type="city">Fribourg-en-Brisgau</settlement></placeName></affiliation></author><author><name sortKey="Zimmermann, Birger" uniqKey="Zimmermann B">Birger Zimmermann</name><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstrasse 2</s1><s2>79110 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Bade-Wurtemberg</region><region type="district" nuts="2">District de Fribourg-en-Brisgau</region><settlement type="city">Fribourg-en-Brisgau</settlement></placeName></affiliation></author><author><name sortKey="W Rfel, Uli" uniqKey="W Rfel U">Uli W Rfel</name><affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Freiburg Materials Research Center (FMF), Stefan-Meier-Strasse 21</s1><s2>79104 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Bade-Wurtemberg</region><region type="district" nuts="2">District de Fribourg-en-Brisgau</region><settlement type="city">Fribourg-en-Brisgau</settlement></placeName></affiliation><affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstrasse 2</s1><s2>79110 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>Allemagne</country><placeName><region type="land" nuts="1">Bade-Wurtemberg</region><region type="district" nuts="2">District de Fribourg-en-Brisgau</region><settlement type="city">Fribourg-en-Brisgau</settlement></placeName></affiliation></author></titleStmt><publicationStmt><idno type="inist">13-0303789</idno><date when="2013">2013</date><idno type="stanalyst">PASCAL 13-0303789 INIST</idno><idno type="RBID">Pascal:13-0303789</idno><idno type="wicri:Area/Main/Corpus">000758</idno><idno type="wicri:Area/Main/Repository">000A11</idno></publicationStmt><seriesStmt><idno type="ISSN">0927-0248</idno><title level="j" type="abbreviated">Sol. energy mater. sol. cells</title><title level="j" type="main">Solar energy materials and solar cells</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Aluminium addition</term><term>Aluminium oxide</term><term>Bearing(mechanics)</term><term>Compatibility</term><term>Conversion rate</term><term>Cost lowering</term><term>Energy conversion</term><term>Flexible structure</term><term>Heterojunction</term><term>High efficiency</term><term>High power</term><term>ITO layers</term><term>Indium oxide</term><term>Industrial production</term><term>Manufacturing process</term><term>Organic solar cells</term><term>Polymer blends</term><term>Production process</term><term>Sheet resistivity</term><term>Silver</term><term>Solar cell</term><term>Stacking</term><term>Styrenesulfonate polymer</term><term>Thin film</term><term>Thiophene derivative polymer</term><term>Tin addition</term><term>Transparent material</term><term>Zinc oxide</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Addition étain</term><term>Cellule solaire organique</term><term>Rendement élevé</term><term>Grande puissance</term><term>Conversion énergie</term><term>Taux conversion</term><term>Palier</term><term>Couche ITO</term><term>Production industrielle</term><term>Processus fabrication</term><term>Procédé fabrication</term><term>Structure flexible</term><term>Diminution coût</term><term>Empilement</term><term>Addition aluminium</term><term>Cellule solaire</term><term>Hétérojonction</term><term>Résistivité couche</term><term>Compatibilité</term><term>Oxyde d'indium</term><term>Styrènesulfonate polymère</term><term>Thiophène dérivé polymère</term><term>Mélange polymère</term><term>Oxyde d'aluminium</term><term>Oxyde de zinc</term><term>Couche mince</term><term>Argent</term><term>Matériau transparent</term><term>ITO</term></keywords><keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Production industrielle</term><term>Argent</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Highest published power conversion efficiencies of organic solar cells have mostly been achieved on substrates bearing a transparent indium tin oxide (ITO) electrode. However, the incorporation of ITO is not suited for future industrial production processes of organic solar cells, which will rely on a high-throughput of flexible substrates in order to achieve low cost of the final product. In this manuscript we present an alternative transparent electrode consisting of a layer stack of aluminum doped zinc oxide and a thin silver layer. Substrates with these electrodes have a transparency of above 75% in the wavelength range in which the photoactive layer absorbs light. Solar cells with a bulk-heterojunction of PTB7 and PC<sub>71</sub>BM in an inverted device architecture achieved a power conversion efficiency of 6.1%, which is the highest reported value for polymer solar cells free from both ITO and PEDOT:PSS. The sheet resistance of the novel electrodes increased only marginally after repeated bending which shows their full compatibility with future reel-to-reel processes or flexible products.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0927-0248</s0></fA01><fA03 i2="1"><s0>Sol. energy mater. sol. cells</s0></fA03><fA05><s2>117</s2></fA05><fA08 i1="01" i2="1" l="ENG"><s1>Inverted ITO- and PEDOT:PSS-free polymer solar cells with high power conversion efficiency</s1></fA08><fA11 i1="01" i2="1"><s1>KOHLSTÄDT (Markus)</s1></fA11><fA11 i1="02" i2="1"><s1>GREIN (Maria)</s1></fA11><fA11 i1="03" i2="1"><s1>REINECKE (Patrick)</s1></fA11><fA11 i1="04" i2="1"><s1>KROYER (Thomas)</s1></fA11><fA11 i1="05" i2="1"><s1>ZIMMERMANN (Birger)</s1></fA11><fA11 i1="06" i2="1"><s1>WÜRFEL (Uli)</s1></fA11><fA14 i1="01"><s1>Freiburg Materials Research Center (FMF), Stefan-Meier-Strasse 21</s1><s2>79104 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>3 aut.</sZ><sZ>6 aut.</sZ></fA14><fA14 i1="02"><s1>Fraunhofer Institute for Solar Energy Systems (ISE), Heidenhofstrasse 2</s1><s2>79110 Freiburg</s2><s3>DEU</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></fA14><fA20><s1>98-102</s1></fA20><fA21><s1>2013</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>18016</s2><s5>354000501971110160</s5></fA43><fA44><s0>0000</s0><s1>© 2013 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>72 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>13-0303789</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Solar energy materials and solar cells</s0></fA64><fA66 i1="01"><s0>NLD</s0></fA66><fC01 i1="01" l="ENG"><s0>Highest published power conversion efficiencies of organic solar cells have mostly been achieved on substrates bearing a transparent indium tin oxide (ITO) electrode. However, the incorporation of ITO is not suited for future industrial production processes of organic solar cells, which will rely on a high-throughput of flexible substrates in order to achieve low cost of the final product. In this manuscript we present an alternative transparent electrode consisting of a layer stack of aluminum doped zinc oxide and a thin silver layer. Substrates with these electrodes have a transparency of above 75% in the wavelength range in which the photoactive layer absorbs light. Solar cells with a bulk-heterojunction of PTB7 and PC<sub>71</sub>BM in an inverted device architecture achieved a power conversion efficiency of 6.1%, which is the highest reported value for polymer solar cells free from both ITO and PEDOT:PSS. The sheet resistance of the novel electrodes increased only marginally after repeated bending which shows their full compatibility with future reel-to-reel processes or flexible products.</s0></fC01><fC02 i1="01" i2="X"><s0>001D06C02D1</s0></fC02><fC02 i1="02" i2="X"><s0>001D05I03D</s0></fC02><fC02 i1="03" i2="X"><s0>230</s0></fC02><fC03 i1="01" i2="X" l="FRE"><s0>Addition étain</s0><s5>01</s5></fC03><fC03 i1="01" i2="X" l="ENG"><s0>Tin addition</s0><s5>01</s5></fC03><fC03 i1="01" i2="X" l="SPA"><s0>Adición estaño</s0><s5>01</s5></fC03><fC03 i1="02" i2="3" l="FRE"><s0>Cellule solaire organique</s0><s5>02</s5></fC03><fC03 i1="02" i2="3" l="ENG"><s0>Organic solar cells</s0><s5>02</s5></fC03><fC03 i1="03" i2="X" l="FRE"><s0>Rendement élevé</s0><s5>03</s5></fC03><fC03 i1="03" i2="X" l="ENG"><s0>High efficiency</s0><s5>03</s5></fC03><fC03 i1="03" i2="X" l="SPA"><s0>Rendimiento elevado</s0><s5>03</s5></fC03><fC03 i1="04" i2="X" l="FRE"><s0>Grande puissance</s0><s5>04</s5></fC03><fC03 i1="04" 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l="ENG"><s0>Industrial production</s0><s5>09</s5></fC03><fC03 i1="09" i2="X" l="SPA"><s0>Producción industrial</s0><s5>09</s5></fC03><fC03 i1="10" i2="X" l="FRE"><s0>Processus fabrication</s0><s5>10</s5></fC03><fC03 i1="10" i2="X" l="ENG"><s0>Production process</s0><s5>10</s5></fC03><fC03 i1="10" i2="X" l="SPA"><s0>Proceso fabricación</s0><s5>10</s5></fC03><fC03 i1="11" i2="X" l="FRE"><s0>Procédé fabrication</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="ENG"><s0>Manufacturing process</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="SPA"><s0>Procedimiento fabricación</s0><s5>11</s5></fC03><fC03 i1="12" i2="X" l="FRE"><s0>Structure flexible</s0><s5>12</s5></fC03><fC03 i1="12" i2="X" l="ENG"><s0>Flexible structure</s0><s5>12</s5></fC03><fC03 i1="12" i2="X" l="SPA"><s0>Estructura flexible</s0><s5>12</s5></fC03><fC03 i1="13" i2="X" l="FRE"><s0>Diminution coût</s0><s5>13</s5></fC03><fC03 i1="13" i2="X" l="ENG"><s0>Cost lowering</s0><s5>13</s5></fC03><fC03 i1="13" i2="X" l="SPA"><s0>Reducción 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resistivity</s0><s5>18</s5></fC03><fC03 i1="18" i2="X" l="SPA"><s0>Resistividad capa</s0><s5>18</s5></fC03><fC03 i1="19" i2="X" l="FRE"><s0>Compatibilité</s0><s5>19</s5></fC03><fC03 i1="19" i2="X" l="ENG"><s0>Compatibility</s0><s5>19</s5></fC03><fC03 i1="19" i2="X" l="SPA"><s0>Compatibilidad</s0><s5>19</s5></fC03><fC03 i1="20" i2="X" l="FRE"><s0>Oxyde d'indium</s0><s5>22</s5></fC03><fC03 i1="20" i2="X" l="ENG"><s0>Indium oxide</s0><s5>22</s5></fC03><fC03 i1="20" i2="X" l="SPA"><s0>Indio óxido</s0><s5>22</s5></fC03><fC03 i1="21" i2="X" l="FRE"><s0>Styrènesulfonate polymère</s0><s2>NK</s2><s5>23</s5></fC03><fC03 i1="21" i2="X" l="ENG"><s0>Styrenesulfonate polymer</s0><s2>NK</s2><s5>23</s5></fC03><fC03 i1="21" i2="X" l="SPA"><s0>Estireno sulfonato polímero</s0><s2>NK</s2><s5>23</s5></fC03><fC03 i1="22" i2="X" l="FRE"><s0>Thiophène dérivé polymère</s0><s2>NK</s2><s5>24</s5></fC03><fC03 i1="22" i2="X" l="ENG"><s0>Thiophene derivative polymer</s0><s2>NK</s2><s5>24</s5></fC03><fC03 i1="22" i2="X" l="SPA"><s0>Tiofeno derivado polímero</s0><s2>NK</s2><s5>24</s5></fC03><fC03 i1="23" i2="3" l="FRE"><s0>Mélange polymère</s0><s5>25</s5></fC03><fC03 i1="23" i2="3" l="ENG"><s0>Polymer blends</s0><s5>25</s5></fC03><fC03 i1="24" i2="X" l="FRE"><s0>Oxyde d'aluminium</s0><s5>26</s5></fC03><fC03 i1="24" i2="X" l="ENG"><s0>Aluminium oxide</s0><s5>26</s5></fC03><fC03 i1="24" i2="X" l="SPA"><s0>Aluminio óxido</s0><s5>26</s5></fC03><fC03 i1="25" i2="X" l="FRE"><s0>Oxyde de zinc</s0><s5>27</s5></fC03><fC03 i1="25" i2="X" l="ENG"><s0>Zinc oxide</s0><s5>27</s5></fC03><fC03 i1="25" i2="X" l="SPA"><s0>Zinc óxido</s0><s5>27</s5></fC03><fC03 i1="26" i2="X" l="FRE"><s0>Couche mince</s0><s5>28</s5></fC03><fC03 i1="26" i2="X" l="ENG"><s0>Thin film</s0><s5>28</s5></fC03><fC03 i1="26" i2="X" l="SPA"><s0>Capa fina</s0><s5>28</s5></fC03><fC03 i1="27" i2="X" l="FRE"><s0>Argent</s0><s2>NC</s2><s2>FX</s2><s5>29</s5></fC03><fC03 i1="27" i2="X" l="ENG"><s0>Silver</s0><s2>NC</s2><s2>FX</s2><s5>29</s5></fC03><fC03 i1="27" i2="X" l="SPA"><s0>Plata</s0><s2>NC</s2><s2>FX</s2><s5>29</s5></fC03><fC03 i1="28" i2="X" l="FRE"><s0>Matériau transparent</s0><s5>30</s5></fC03><fC03 i1="28" i2="X" l="ENG"><s0>Transparent material</s0><s5>30</s5></fC03><fC03 i1="28" i2="X" l="SPA"><s0>Material transparente</s0><s5>30</s5></fC03><fC03 i1="29" i2="X" l="FRE"><s0>ITO</s0><s4>INC</s4><s5>82</s5></fC03><fN21><s1>287</s1></fN21><fN44 i1="01"><s1>OTO</s1></fN44><fN82><s1>OTO</s1></fN82></pA></standard></inist></record>Pour manipuler ce document sous Unix (Dilib)
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